Four councils in outer London say the scheme will his its poorest residents most.
Now Hillingdon, Harrow, Bexley and Croydon councils have announced their opposition to the widening of the zone.
"Unlike urban parts of the capital, our residents don't have the luxury of a frequent, multi-layered transport system. London Borough of Bexley leader Baroness O'Neill said: "We are an outer London borough with poor transport connections, which means that many people are reliant on their cars, including many who travel into the borough from outside London.
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